The National Academies of Sciences, Engineering, and Medicine organized a workshop to discuss the usefulness of the classified observing systems in advancing understanding of cloud and aerosol interactions. Because these systems were not developed with weather and climate modeling as a primary mission objective, many participants said it is necessary for scientists to find creative ways to utilize the data. The data from these systems have the potential to be useful in advancing understanding of cloud and aerosol interactions. This publication summarizes the presentations and discussions from the workshop.